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Is there a way to configure Outlook 2007 so by pressing a [CTRL]+[letter] combination, a macro is activated?

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did you find a solution? I'm having the same problem and it is really a pity if that should be impossible. – MostlyHarmless Jan 17 '13 at 8:24

This MSDN blog post shows how you can add macros to the toolbar then use an Alt keyboard shortcut to access them.

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