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I've been switching keyboard layouts in Windows with Alt+Shift. But I want to do it with a single key only (such as ctrl). Is it possible?

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Ctrl is usually taken as a modifier, not as a key.

But you may use a macro product like AutoHotkey, to define a macro that translates one of your Ctrl keys to Alt+Shift.

Or it might be easier to use a keyboard-mapping product such as SharpKeys or KeyTweak :

image

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