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I have a laptop with Pop!_OS installed and I don't want to partition or touch that hard drive at all since it is my main work machine. I installed a second hard drive and put Windows 10 on it, so the machine is now dual-booting on two separate hard drives.

Next, I'd love to virtualize the Windows 10 installation inside Pop!_OS. I created a vmdk that points to the SSD I installed Windows 10 on and created a machine but I get a "No bootable medium found!". I also used VBoxManage storageattach "Windows 10" --storagectl "SATA" --port 0 --device 0 --type hdd --medium ~/VirtualBox\ VMs/win10.vmdk to attach the drive, but it still gives me the same error.

I'm not sure if it means anything or not but gparted shows two partitions that seem suspect labeled "boot/efi" and "msftdata" on my main Linux partition:

GParted partition table

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If I understand right, you have installed Windows in a situation of dual boot on your main disk and would now like to move Windows into a vmdk. This was not the right way to achieve that.

My guess is that your boot device is the first disk, so the Windows disk has no boot capabilities by itself - you boot it through the first disk.

I suggest to set on the VM a Windows ISO as boot device, and re-install Windows while running from the virtual product (VMware?). You could probably get by doing only a Startup Repair rather than a full installation of Windows 10.

I suggest before starting to undo the dual boot, since after the above is finished I'm not sure that the dual boot will still work.

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